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Properties of Ag-doped Bi-Sb alloys as thermoelectric conversion materials for solid state refrigeration

Wen XU, Laifeng LI, Rongjin HUANG, Min ZHOU, Liyun ZHENG, Linghui GONG, Chunmei SONG

《能源前沿（英文）》 2009年 第3卷 第1期   页码 90-93 doi: 10.1007/s11708-009-0005-1

摘要： The energy conversion properties of Bi-Sb system thermoelectric materials doped by Ag was investigated. Bi Sb Ag ( =0, 1, 2, 3, 4) alloys with Ag substitution for Sb were synthesized by mechanical alloying and then pressed under 5 GPa at 523 K for 30 min. The phase structure of the alloys was characterized by X-ray diffraction. The electric conductivities and the seebeck coefficients were measured at the temperature range of 80-300 K. The results reveal that the electric conductivities of the Ag-doped Bi-Sb alloys are highly improved. The power factor of Bi Sb Ag reaches a maximum value of 2.98×10 W/(K ?m) at 255 K, which is about three times that of the un-doped sample Bi Sb at the same temperature.

关键词： thermoelectric conversion materials     high-pressure sintering     thermoelectric properties    

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A thermoelectric generator and water-cooling assisted high conversion efficiency polycrystalline silicon

Zekun LIU, Shuang YUAN, Yi YUAN, Guojian LI, Qiang WANG

《能源前沿（英文）》 2021年 第15卷 第2期   页码 358-366 doi: 10.1007/s11708-020-0712-1

摘要： Solar energy has been increasing its share in the global energy structure. However, the thermal radiation brought by sunlight will attenuate the efficiency of solar cells. To reduce the temperature of the photovoltaic (PV) cell and improve the utilization efficiency of solar energy, a hybrid system composed of the PV cell, a thermoelectric generator (TEG), and a water-cooled plate (WCP) was manufactured. The WCP cannot only cool the PV cell, but also effectively generate additional electric energy with the TEG using the waste heat of the PV cell. The changes in the efficiency and power density of the hybrid system were obtained by real time monitoring. The thermal and electrical tests were performed at different irradiations and the same experiment temperature of 22°C. At a light intensity of 1000 W/m , the steady-state temperature of the PV cell decreases from 86.8°C to 54.1°C, and the overall efficiency increases from 15.6% to 21.1%. At a light intensity of 800 W/m , the steady-state temperature of the PV cell decreases from 70°C to 45.8°C, and the overall efficiency increases from 9.28% to 12.59%. At a light intensity of 400 W/m , the steady-state temperature of the PV cell decreases from 38.5°C to 31.5°C, and the overall efficiency is approximately 3.8%, basically remain unchanged.

关键词： photovoltaic (PV)     thermoelectric generator     conversion efficiency     hybrid energy systems     water-cooled plate (WCP)    

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Developments in semiconductor thermoelectric materials

Laifeng LI, Zhen CHEN, Min ZHOU, Rongjin HUANG

《能源前沿（英文）》 2011年 第5卷 第2期   页码 125-136 doi: 10.1007/s11708-011-0150-1

摘要： A surge in interest in developing alternative renewable energy technologies has been observed in recent years. In particular, thermoelectrics has drawn attention because thermoelectric effects enable direct conversion between thermal and electrical energy, and provide power generation and refrigeration alternatives. During the past decade, the performance of thermoelectric materials has been considerably improved; however, many challenges continue to exist. Developing thermoelectric materials with superior performance means tailoring interconnected thermoelectric physical parameters-electrical conductivities, Seebeck coefficients, and thermal conductivities for a crystalline system. The objectives of this paper are to introduce the recent developments in semiconductor thermoelectric materials, and briefly summarize the applications of such materials.

关键词： thermoelectric materials     thermoelectric figure of merit     applications    

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Nanostructural thermoelectric materials and their performance

Kai-Xuan CHEN, Min-Shan LI, Dong-Chuan MO, Shu-Shen LYU

《能源前沿（英文）》 2018年 第12卷 第1期   页码 97-108 doi: 10.1007/s11708-018-0543-5

摘要： In this review, an attempt was made to introduce the traditional concepts and materials in thermoelectric application and the recent development in searching high-performance thermoelectric materials. Due to the use of nanostructural engineering, thermoelectric materials with a high figure of merit are designed, leading to their blooming application in the energy field. One dimensional nanotubes and nanoribbons, two-dimensional planner structures, nanocomposites, and heterostructures were summarized. In addition, the state-of-the-art theoretical calculation in the prediction of thermoelectric materials was also reviewed, including the molecular dynamics (MD), Boltzmann transport equation, and non-equilibrium Green’s function. The combination of experimental fabrication and first-principles prediction significantly promotes the discovery of new promising candidates in the thermoelectric field.

关键词： nanostructural     low-dimensional     thermoelectric material     figure of merit     first-principles    

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Near-field radiative thermoelectric energy converters: a review

Eric TERVO, Elham BAGHERISERESHKI, Zhuomin ZHANG

《能源前沿（英文）》 2018年 第12卷 第1期   页码 5-21 doi: 10.1007/s11708-017-0517-z

摘要： Radiative thermoelectric energy converters, which include thermophotovoltaic cells, thermoradiative cells, electroluminescent refrigerators, and negative electroluminescent refrigerators, are semiconductor p-n devices that either generate electricity or extract heat from a cold body while exchanging thermal radiation with their surroundings. If this exchange occurs at micro or nanoscale distances, power densities can be greatly enhanced and near-field radiation effects may improve performance. This review covers the fundamentals of near-field thermal radiation, photon entropy, and nonequilibrium effects in semiconductor diodes that underpin device operation. The development and state of the art of these near-field converters are discussed in detail, and remaining challenges and opportunities for progress are identified.

关键词： energy conversion systems     luminescent refrigeration     near-field radiation     thermophotovoltaic     thermoradiative cell    

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High performance solid-state thermoelectric energy conversion via inorganic metal halide perovskites

Lifu YAN, Lingling ZHAO, Guiting YANG, Shichao LIU, Yang LIU, Shangchao LIN

《能源前沿（英文）》 2022年 第16卷 第4期   页码 581-594 doi: 10.1007/s11708-022-0831-y

摘要： Solid-state thermoelectric energy conversion devices attract broad research interests because of their great promises in waste heat recycling, space power generation, deep water power generation, and temperature control, but the search for essential thermoelectric materials with high performance still remains a great challenge. As an emerging low cost, solution-processed thermoelectric material, inorganic metal halide perovskites CsPb(I1–xBrx)3 under mechanical deformation is systematically investigated using the first-principle calculations and the Boltzmann transport theory. It is demonstrated that halogen mixing and mechanical deformation are efficient methods to tailor electronic structures and charge transport properties in CsPb(I1–xBrx)3 synergistically. Halogen mixing leads to band splitting and anisotropic charge transport due to symmetry-breaking-induced intrinsic strains. Such band splitting reconstructs the band edge and can decrease the charge carrier effective mass, leading to excellent charge transport properties. Mechanical deformation can further push the orbital energies apart from each other in a more controllable manner, surpassing the impact from intrinsic strains. Both anisotropic charge transport properties andZT values are sensitive to the direction and magnitude of strain, showing a wide range of variation from 20% to 400% (with a ZT value of up to 1.85) compared with unstrained cases. The power generation efficiency of the thermoelectric device can reach as high as approximately 12% using mixed halide perovskites under tailored mechanical deformation when the heat-source is at 500 K and the cold side is maintained at 300 K, surpassing the performance of many existing bulk thermoelectric materials.

关键词： inorganic metal halide perovskites     mechanical deformation     thermoelectrics     first-principle calculations     Boltzmann transport theory    

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Clean energy technology: materials, processes and devices for electrochemical energy conversion and storage

Hong YANG, Junliang ZHANG, Baolian YI

《能源前沿（英文）》 2017年 第11卷 第3期   页码 233-235 doi: 10.1007/s11708-017-0501-7

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Recent development and application of thin-film thermoelectric cooler

Yuedong Yu, Wei Zhu, Xixia Kong, Yaling Wang, Pengcheng Zhu, Yuan Deng

《化学科学与工程前沿（英文）》 2020年 第14卷 第4期   页码 492-503 doi: 10.1007/s11705-019-1829-9

摘要： Recently, the performance and fabrication of thin-film thermoelectric materials have been largely enhanced. Based on this enhancement, the thin-film thermoelectric cooler (TEC) is becoming a research hot topic, due to its high cooling flux and microchip level size. To fulfill a thin-film TEC, interfacial problems are unavoidable, as they may largely reduce the properties of a thin-film TEC. Moreover, the architecture of a thin-film TEC should also be properly designed. In this review, we introduced the enhancement of thermoelectric properties of (Bi,Sb) (Te,Se) solid solution materials by chemical vapor deposition, physical vapor deposition and electrodeposition. Then, the interfacial problems, including contact resistance, interfacial diffusion and thermal contact resistance, were discussed. Furthermore, the design, fabrication, as well as the performance of thin-film TECs were summarized.

关键词： thin-film thermoelectric cooler     interfaces     cooling flux     TE device fabrication    

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Photothermal materials for efficient solar powered steam generation

Fenghua Liu, Yijian Lai, Binyuan Zhao, Robert Bradley, Weiping Wu

《化学科学与工程前沿（英文）》 2019年 第13卷 第4期   页码 636-653 doi: 10.1007/s11705-019-1824-1

摘要： Solar powered steam generation is an emerging area in the field of energy harvest and sustainable technologies. The nano-structured photothermal materials are able to harvest energy from the full solar spectrum and convert it to heat with high efficiency. Moreover, the materials and structures for heat management as well as the mass transportation are also brought to the forefront. Several groups have reported their materials and structures as solutions for high performance devices, a few creatively coupled other physical fields with solar energy to achieve even better results. This paper provides a systematic review on the recent developments in photothermal nanomaterial discovery, material selection, structural design and mass/heat management, as well as their applications in seawater desalination and fresh water production from waste water with free solar energy. It also discusses current technical challenges and likely future developments. This article will help to stimulate novel ideas and new designs for the photothermal materials, towards efficient, low cost practical solar-driven clean water production.

关键词： solar stream generation     plasmonics     porous carbon     photothermal materials     solar energy conversion efficiency     water vapor generation rate    

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polyethylene glycol in cellulose-based porous capsules for latent heat storage and light-to-thermal conversion

《化学科学与工程前沿（英文）》 2023年 第17卷 第8期   页码 1038-1050 doi: 10.1007/s11705-022-2279-3

摘要： Phase change materials are potential candidates for the application of latent heat storage. Herein, we fabricated porous capsules as shape-stable materials from cellulose-based polyelectrolyte complex, which were first prepared using cellulose 6-(N-pyridinium)hexanoyl ester as the cationic polyelectrolyte and carboxymethyl cellulose as the anionic polyelectrolyte to encapsulate polyethylene glycol by the vacuum impregnation method. Furthermore, the multi-walled carbon nanotube or graphene oxide, which were separately composited into the polyelectrolytes complex capsules to enhance thermal conductivity and light-to-thermal conversion efficiency. These capsules owned a typical core–shell structure, with an extremely high polyethylene glycol loading up to 34.33 g∙g‒1. After loading of polyethylene glycol, the resulted cellulose-based composite phase change materials exhibited high thermal energy storage ability with the latent heat up to 142.2 J∙g‒1, which was 98.5% of pure polyethylene glycol. Further results showed that the composite phase change materials demonstrated good form-stable property and thermal stability. Moreover, studies involving light-to-thermal conversion determined that composite phase change materials exhibited outstanding light-to-thermal conversion performance. Considering their exceptional comprehensive features, innovative composite phase change materials generated from cellulose presented a highly interesting choice for thermal management and renewable thermal energy storage.

关键词： cellulose     polyelectrolytes     phase change materials     thermal energy storage     light-to-thermal conversion    

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MEMS-based thermoelectric infrared sensors: A review

Dehui XU, Yuelin WANG, Bin XIONG, Tie LI

《机械工程前沿（英文）》 2017年 第12卷 第4期   页码 557-566 doi: 10.1007/s11465-017-0441-2

摘要：

In the past decade, micro-electromechanical systems (MEMS)-based thermoelectric infrared (IR) sensors have received considerable attention because of the advances in micromachining technology. This paper presents a review of MEMS-based thermoelectric IR sensors. The first part describes the physics of the device and discusses the figures of merit. The second part discusses the sensing materials, thermal isolation microstructures, absorber designs, and packaging methods for these sensors and provides examples. Moreover, the status of sensor implementation technology is examined from a historical perspective by presenting findings from the early years to the most recent findings.

关键词： thermoelectric infrared sensor     CMOS-MEMS     thermopile     micromachining     wafer-level package    

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Evaluation of the power-generation capacity of wearable thermoelectric power generator

Yang YANG, Jing LIU,

《能源前沿（英文）》 2010年 第4卷 第3期   页码 346-357 doi: 10.1007/s11708-010-0112-z

摘要： Employing thermoelectric generators (TEGs) to gather heat dissipating from the human body through the skin surface is a promising way to supply electronic power to wearable and pocket electronics. The uniqueness of this method lies in its direct utilization of the temperature difference between the environment and the human body, and complete elimination of power maintenance problems. However, most of the previous investigations on thermal energy harvesters are confined to the TEG and electronic system themselves because of the low quality of human energy. We evaluate the energy generation capacity of a wearable TEG subject to various conditions based on biological heat transfer theory. Through numerical simulation and corresponding parametric studies, we find that the temperature distribution in the thermopiles affects the criterion of the voltage output, suggesting that the temperature difference in a single point can be adopted as the criterion for uniform temperature distribution. However, the criterion has to be shifted to the sum of temperature difference on each thermocouple when the temperature distribution is inconsistent. In addition, the performance of the thermal energy harvester can be easily influenced by environmental conditions, as well as the physiological state and physical characteristics of the human body. To further validate the calculation results for the wearable TEG, a series of conceptual experiments are performed on a number of typical cases. The numerical simulation provides a good overview of the electricity generation capability of the TEG, which may prove useful in the design of future thermal energy harvesters.

关键词： thermal energy harvester     thermoelectric generator     biological heat transfer     power generating capacity    

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Effect of non-uniform illumination on performance of solar thermoelectric generators

Ershuai YIN, Qiang LI, Yimin XUAN

《能源前沿（英文）》 2018年 第12卷 第2期   页码 239-248 doi: 10.1007/s11708-018-0533-7

摘要： Solar thermoelectric generators (STEGs) are heat engines which can generate electricity from concentrated sunlight. The non-uniform illumination caused by the optical concentrator may affect the performance of solar thermoelectric generators. In this paper, a three-dimensional finite element model of solar thermoelectric generators is established. The two-dimensional Gaussian distribution is employed to modify the illumination profiles incident on the thermoelectric generator. Six non-uniformities of solar illumination are investigated while keeping the total energy constant. The influences of non-uniform illumination on the temperature distribution, the voltage distribution, and the maximum output power are respectively discussed. Three thermoelectric generators with 32, 18 and 8 pairs of thermocouples are compared to investigate their capability under non-uniform solar radiation. The result shows that the non-uniformity of the solar illumination has a great effect on the temperature distribution and the voltage distribution. Central thermoelectric legs can achieve a larger temperature difference and generate a larger voltage than peripheral ones. The non-uniform solar illumination will weaken the capability of the TE generator, and the maximum output power decrease by 1.4% among the range of non-uniformity studied in this paper. Reducing the number of the thermoelectric legs for non-uniform solar illumination can greatly increase the performance of the thermoelectric generator.

关键词： solar thermoelectric generators     non-uniform solar illumination     performance evaluation     solar energy    

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温差发电的热力过程研究及材料的塞贝克系数测定

贾磊,胡芃,陈则韶

《中国工程科学》 2005年 第7卷 第12期   页码 31-34

摘要：

建立了半导体温差发电器件的基本模型；从稳态的热传导方程出发，对发电器件进行了热力学分析，推导出P型和N型半导体内部的温度分布函数及输出功率和发电效率的表达式；测定了一种Bi-Te-Sb-Se半导体热电材料在低温下的塞贝克系数随温度的变化关系，绘制了曲线并进行数值拟合；结果表明，该种半导体热电材料在低温下性能不佳，需改进配方或生产工艺方可使用。

关键词： 半导体     温差发电     热力过程     塞贝克系数    

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Multifunctional, Wearable, and Wireless Sensing System via Thermoelectric Fabrics

Xinyang He,Jiaxin Cai,Mingyuan Liu,Xuepeng Ni,Wendi Liu,Hanyu Guo,Jianyong Yu,Liming Wang,Xiaohong Qin,

《工程（英文）》 doi: 10.1016/j.eng.2023.05.026

摘要： Flexible thermoelectric materials play an important role in smart wearables, such as wearable power generation, self-powered sensing, and personal thermal management. However, with the rapid development of Internet of Things (IoT) and artificial intelligence (AI), higher standards for comfort, multifunctionality, and sustainable operation of wearable electronics have been proposed, and it remains challenging to meet all the requirements of currently reported thermoelectric devices. Herein, we present a multifunctional, wearable, and wireless sensing system based on a thermoelectric knitted fabric with over 600 mm·s−1 air permeability and a stretchability of 120%. The device coupled with a wireless transmission system realizes self-powered monitoring of human respiration through an mobile phone application (APP). Furthermore, an integrated thermoelectric system was designed to combine photothermal conversion and passive radiative cooling, enabling the characteristics of being powered by solar-driven in-plane temperature differences and monitoring outdoor sunlight intensity through the APP. Additionally, we decoupled the complex signals of resistance and thermal voltage during deformation under solar irradiation based on the anisotropy of the knitted fabrics to enable the device to monitor and optimize the outdoor physical activity of the athlete via the APP. This novel thermoelectric fabric-based wearable and wireless sensing platform has promising applications in next-generation smart textiles.

关键词： Thermoelectric fabrics     Wearable device     Wireless     Multifunctional sensing system     Outdoor wearable signal monitoring    

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标题 作者 时间 类型 操作

Properties of Ag-doped Bi-Sb alloys as thermoelectric conversion materials for solid state refrigeration

Wen XU, Laifeng LI, Rongjin HUANG, Min ZHOU, Liyun ZHENG, Linghui GONG, Chunmei SONG

期刊论文

A thermoelectric generator and water-cooling assisted high conversion efficiency polycrystalline silicon

Zekun LIU, Shuang YUAN, Yi YUAN, Guojian LI, Qiang WANG

期刊论文

Developments in semiconductor thermoelectric materials

Laifeng LI, Zhen CHEN, Min ZHOU, Rongjin HUANG

期刊论文

Nanostructural thermoelectric materials and their performance

Kai-Xuan CHEN, Min-Shan LI, Dong-Chuan MO, Shu-Shen LYU

期刊论文

Near-field radiative thermoelectric energy converters: a review

Eric TERVO, Elham BAGHERISERESHKI, Zhuomin ZHANG

期刊论文

High performance solid-state thermoelectric energy conversion via inorganic metal halide perovskites

Lifu YAN, Lingling ZHAO, Guiting YANG, Shichao LIU, Yang LIU, Shangchao LIN

期刊论文

Clean energy technology: materials, processes and devices for electrochemical energy conversion and storage

Hong YANG, Junliang ZHANG, Baolian YI

期刊论文

Recent development and application of thin-film thermoelectric cooler

Yuedong Yu, Wei Zhu, Xixia Kong, Yaling Wang, Pengcheng Zhu, Yuan Deng

期刊论文

Photothermal materials for efficient solar powered steam generation

Fenghua Liu, Yijian Lai, Binyuan Zhao, Robert Bradley, Weiping Wu

期刊论文

polyethylene glycol in cellulose-based porous capsules for latent heat storage and light-to-thermal conversion

期刊论文

MEMS-based thermoelectric infrared sensors: A review

Dehui XU, Yuelin WANG, Bin XIONG, Tie LI

期刊论文

Evaluation of the power-generation capacity of wearable thermoelectric power generator

Yang YANG, Jing LIU,

期刊论文

Effect of non-uniform illumination on performance of solar thermoelectric generators

Ershuai YIN, Qiang LI, Yimin XUAN

期刊论文

温差发电的热力过程研究及材料的塞贝克系数测定

贾磊,胡芃,陈则韶

期刊论文

Multifunctional, Wearable, and Wireless Sensing System via Thermoelectric Fabrics

Xinyang He,Jiaxin Cai,Mingyuan Liu,Xuepeng Ni,Wendi Liu,Hanyu Guo,Jianyong Yu,Liming Wang,Xiaohong Qin,

期刊论文